Strong angular and spectral narrowing of electroluminescence in an integrated Tamm-plasmon-driven halide perovskite LED

集成 Tamm 等离子体驱动卤化物钙钛矿 LED 中电致发光的强烈角度和光谱窄化

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作者:Zher Ying Ooi, Alberto Jiménez-Solano, Krzysztof Gałkowski, Yuqi Sun, Jordi Ferrer Orri, Kyle Frohna, Hayden Salway, Simon Kahmann, Shenyu Nie, Guadalupe Vega, Shaoni Kar, Michał P Nowak, Sebastian Maćkowski, Piotr Nyga, Caterina Ducati, Neil C Greenham, Bettina V Lotsch, Miguel Anaya, Samuel D Stra

Abstract

Next-generation light-emitting applications such as displays and optical communications require judicious control over emitted light, including intensity and angular dispersion. To date, this remains a challenge as conventional methods require cumbersome optics. Here, we report highly directional and enhanced electroluminescence from a solution-processed quasi-2-dimensional halide perovskite light-emitting diode by building a device architecture to exploit hybrid plasmonic-photonic Tamm plasmon modes. By exploiting the processing and bandgap tunability of the halide perovskite device layers, we construct the device stack to optimise both optical and charge-injection properties, leading to narrow forward electroluminescence with an angular full-width half-maximum of 36.6° compared with the conventional isotropic control device of 143.9°, and narrow electroluminescence spectral full-width half-maximum of 12.1 nm. The device design is versatile and tunable to work with emission lines covering the visible spectrum with desired directionality, thus providing a promising route to modular, inexpensive, and directional operating light-emitting devices.

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