Two-dimensional double-quantum spectra reveal collective resonances in an atomic vapor

二维双量子光谱揭示了原子蒸气中的集体共振

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Abstract

We report the observation of double-quantum coherence signals in a gas of potassium atoms at twice the frequency of the one-quantum coherences. Since a single atom does not have a state at the corresponding energy, this observation must be attributed to a collective resonance involving multiple atoms. These resonances are induced by weak interatomic dipole-dipole interactions, which means that the atoms cannot be treated in isolation, even at a low density of 10(12)  cm(-3).

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