Rhodium(I)/diene-catalyzed addition reactions of arylborons with ketones

铑(I)/二烯催化的芳基硼与酮的加成反应

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Abstract

Rh(I)/diene-catalyzed addition reactions of arylboroxines/arylboronic acids with unactivated ketones to form tertiary alcohols in good to excellent yields are described. By using C(2)-symmetric (3aR,6aR)-3,6-diaryl-1,3a,4,6a-tetrahydropentalenes as ligands, the asymmetric version of such an addition reaction, with up to 68% ee, was also realized.

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