A hydrothermally synthesized MoS(2(1-x))Se(2x) alloy with deep-shallow level conversion for enhanced performance of photodetectors

水热合成的MoS(2(1-x))Se(2x)合金具有深浅能级转换特性,可增强光电探测器的性能

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Abstract

Photoelectric detectors based on binary transition metal chalcogenides have attracted widespread attention in recent years. However, due to the high-temperature synthesis of binary TMD, high-density deep-level defect states may be generated, leading to poor responsiveness or a long response time. Besides, the addition of an alloy will change the DLDSs from deep to shallow energy levels caused by S vacancies. In this paper, MoS(2(1-x))Se(2x) nanostructures were synthesized by a hydrothermal method, and a novel type of photodetector was fabricated by using the synthesized material as a light sensitive material. The MoSSe-based photodetector not only has a high photocurrent, but also exhibits a wide spectral response in the range of 405 nm to 808 nm. At the same time, it can achieve a responsivity of 1.753 mA W(-1) under 660 nm laser irradiation of 1.75 mW mm(-2). Therefore, this work can be considered as a method of constructing a new type of photodetector with a simple process and low cost.

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