Electrochemical Hydroboration of Alkynes

炔烃的电化学氢硼化反应

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Abstract

Herein we reported the electrochemical hydroboration of alkynes by using B(2) Pin(2) as the boron source. This unprecedented reaction manifold was applied to a broad range of alkynes, giving the hydroboration products in good to excellent yields without the need of a metal catalyst or a hydride source. This transformation relied on the possible electrochemical oxidation of an in situ formed borate. This anodic oxidation performed in an undivided cell allowed the formation of a putative boryl radical, which reacted on the alkyne.

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