Charge-density waves (CDWs) are ubiquitous in underdoped cuprate superconductors. As a modulation of the valence electron density, CDWs in hole-doped cuprates possess both Cu-3d and O-2p orbital character owing to the strong hybridization of these orbitals near the Fermi level. Here, we investigate underdoped Bi(2)Sr(1.4)La(0.6)CuO(6+δ) using resonant inelastic X-ray scattering (RIXS) and find that a short-range CDW exists at both Cu and O sublattices in the copper-oxide (CuO(2)) planes with a comparable periodicity and correlation length. Furthermore, we uncover bond-stretching and bond-buckling phonon anomalies concomitant to the CDWs. Comparing to slightly overdoped Bi(2)Sr(1.8)La(0.2)CuO(6+δ), where neither CDWs nor phonon anomalies appear, we highlight that a sharp intensity anomaly is induced in the proximity of the CDW wavevector (Q(CDW)) for the bond-buckling phonon, in concert with the diffused intensity enhancement of the bond-stretching phonon at wavevectors much greater than Q(CDW) Our results provide a comprehensive picture of the quasistatic CDWs, their dispersive excitations, and associated electron-phonon anomalies, which are key for understanding the competing electronic instabilities in cuprates.
Multiorbital charge-density wave excitations and concomitant phonon anomalies in Bi(2)Sr(2)LaCuO(6+δ).
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作者:Li Jiemin, Nag Abhishek, Pelliciari Jonathan, Robarts Hannah, Walters Andrew, Garcia-Fernandez Mirian, Eisaki Hiroshi, Song Dongjoon, Ding Hong, Johnston Steven, Comin Riccardo, Zhou Ke-Jin
| 期刊: | Proceedings of the National Academy of Sciences of the United States of America | 影响因子: | 9.100 |
| 时间: | 2020 | 起止号: | 2020 Jul 14; 117(28):16219-16225 |
| doi: | 10.1073/pnas.2001755117 | ||
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