Microwave assisted synthesis and antimicrobial evaluation of novel Thiazolidinedione pyrrole hybrids with antiviral potential and comprehensive computational modeling studies

利用微波辅助合成法制备新型噻唑烷二酮吡咯杂合物,并对其抗菌活性进行评价,同时开展抗病毒活性研究及综合计算建模分析。

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Abstract

A novel class of N-substituted thiazolidine-2,4-dione/pyrrole-2,5-dione moiety derivatives 3(a–g) was synthesized via C–N bond formation through SN(2)-mediated reaction, utilizing microwave-assisted synthesis to enhance reaction efficiency and product yield. This approach enabled the rapid and selective formation of the target compounds, which were evaluated for their in vitro antimicrobial activity against a variety of bacterial and fungal strains. The compounds demonstrated promising antibacterial and antifungal properties, with compound 3g showing the highest activity, producing significant inhibition zones against Gram-negative strains (E. coli and P. aeruginosa) as well as Gram-positive strains (S. aureus and B. subtilis). To further validate and refine the docking outcomes, molecular dynamics (MD) simulations were performed, providing detailed insights into the dynamic stability, conformational adaptability, hydrogen-bond persistence, and overall binding energetics of the most promising ligand–protein complexes. Density functional theory (DFT) calculations provided valuable insights into the electronic properties, stability, and reactivity of the compounds. The study successfully identified targeted compounds exhibiting significant antiviral/anti–SARS-CoV-2 potential using the pharmacophore POM model, highlighting their predicted ability to inhibit crucial viral proteins. The structures of the synthesized compounds were confirmed using a range of spectroscopic techniques, including FT IR, (1)H NMR, (13)C NMR, and mass spectrometry, ensuring the successful synthesis of the bioactive derivatives. SUPPLEMENTARY INFORMATION: The online version contains supplementary material available at 10.1038/s41598-026-39103-4.

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