A Focus on Unusual ECL2 Interactions Yields β(2) -Adrenergic Receptor Antagonists with Unprecedented Scaffolds

聚焦于不寻常的ECL2相互作用,获得了具有前所未有的骨架结构的β(2)-肾上腺素能受体拮抗剂

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Abstract

The binding pockets of aminergic G protein-coupled receptors are often targeted by drugs and virtual screening campaigns. In order to find ligands with unprecedented scaffolds for one of the best-investigated receptors of this subfamily, the β(2) -adrenergic receptor, we conducted a docking-based screen insisting that molecules would address previously untargeted residues in extracellular loop 2. We here report the discovery of ligands with a previously undescribed coumaran-based scaffold. Furthermore, we provide an analysis of the added value that X-ray structures in different conformations deliver for such docking screens.

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