Manganese Complexes Bearing Bulky DAB Ligands as Efficient Catalysts for the Solvent-Free Hydroboration of Ketones

含大体积DAB配体的锰配合物作为高效催化剂用于酮的无溶剂氢硼化反应

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Abstract

Manganese complexes of the general formula [Mn(DAB)(CO)(3)Br] featuring sterically demanding α-diimine ligands (DAB) were prepared, characterized, and found to be catalytically active in the hydroboration of ketones. The developed eco-friendly approach allowed straightforward formation of boronic esters in quantitative yields in mild and solvent-free conditions.

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