Use of a Carbon-ink Microelectrode Array for Signal Enhancement in Microchip Electrophoresis with Electrochemical Detection

利用碳墨微电极阵列增强微芯片电泳信号并进行电化学检测

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Abstract

In this communication, we demonstrate that a carbon ink microelectrode array, where the electrodes are held at the same potential, affords significant signal enhancement in microchip electrophoresis with amperometric detection. The ability to fabricate an array of carbon ink microelectrodes with a palladium decoupler was demonstrated and the resulting electrodes were integrated with a valving microchip design. The use of an 8 electrode array led to a significant improvement in the limits of detection at the expense of separation resolution due to the increased detection zone size. It is also shown that microdialysis sampling can be integrated with the microchip device and a multi-analyte separation achieved.

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