Chitosan Supports Boosting NiCo(2)O(4) for Catalyzed Urea Electrochemical Removal Application

壳聚糖载体增强NiCo(2)O(4)催化尿素电化学去除性能

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Abstract

Currently, wastewater containing high urea levels poses a significant risk to human health. Else, electrocatalytic methodologies have the potential to transform urea present in urea-rich wastewater into hydrogen, thereby contributing towards environmental conservation and facilitating the production of sustainable energy. The characterization of the NiCo(2)O(4)@chitosan catalyst was performed by various analytical techniques, including scanning electron microscopy (SEM) and X-ray photoelectron spectroscopy (XPS). Furthermore, the activity of electrodes toward urea removal was investigated by several electrochemical techniques. As a function of current density, the performance of the modified NiCo(2)O(4)@chitosan surface was employed to remove urea using electrochemical oxidation. Consequently, the current density measurement was 43 mA cm(-2) in a solution of 1.0 M urea and 1.0 M KOH. Different kinetic characteristics were investigated, including charge transfer coefficient (α), Tafel slope (29 mV dec(-1)), diffusion coefficient (1.87 × 10(-5) cm(2) s(-1)), and surface coverage 4.29 × 10(-9) mol cm(-2). The electrode showed high stability whereas it lost 10.4% of its initial current after 5 h of urea oxidation.

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