Synthesis and Characterization of Novel Fe-Mn-Ce Ternary Oxide⁻Biochar Composites as Highly Efficient Adsorbents for As(III) Removal from Aqueous Solutions

新型 Fe-Mn-Ce 三元氧化物⁻生物炭复合材料的合成与表征作为从水溶液中去除 As(III) 的高效吸附剂

阅读:7
作者:Xuewei Liu, Guogang Zhang, Lina Lin, Zulqarnain Haider Khan, Weiwen Qiu, Zhengguo Song

Abstract

The widespread pollution of water bodies with arsenic (As) necessitates the development of efficient decontamination techniques. To address this issue, we herein prepare Fe-Mn-Ce ternary oxide-biochar composites (FMCBCs) using impregnation/sintering methods and examined their physicochemical properties, morphologies, and As(III) removal performances. The specific surface area of FMCBCs increased with increasing Ce content and enhanced the quantity of surface functional groups (⁻OH, ⁻COOH). The adsorption of As(III) on FMCBCs was well represented by pseudo-second-order kinetics, and the As(III) adsorption capacity of the best-performing FMCBCs (8.47 mg g-1 for FMCBC&sub3;) exceeded that of BC by a factor of 2.9. At pH = 3, the amount of adsorption of As(III) by FMCBCs reached a maximum, and the increased ionic strength could enhance adsorption capacity of FMCBCs. Moreover, an As(III) removal efficiency of ~99% was observed for FMCBC&sub3; at a dosage of 8 g L-1, which highlighted its great potential as an absorbent for As(III) removal from contaminated water.

特别声明

1、本页面内容包含部分的内容是基于公开信息的合理引用;引用内容仅为补充信息,不代表本站立场。

2、若认为本页面引用内容涉及侵权,请及时与本站联系,我们将第一时间处理。

3、其他媒体/个人如需使用本页面原创内容,需注明“来源:[生知库]”并获得授权;使用引用内容的,需自行联系原作者获得许可。

4、投稿及合作请联系:info@biocloudy.com。