Sequential Leaching and Mineralogical Controls of Rare Earth Elements and Yttrium Occurrence in Bituminous Coal from Upper Silesian Coal Basin (Poland)

波兰上西里西亚煤盆地烟煤中稀土元素和钇赋存的顺序浸出和矿物学控制

阅读:1

Abstract

In this study, the occurrence and leachability of rare earth elements and yttrium (REY) in medium-rank coal-meta-bituminous B coal from the southwestern part of the Upper Silesian Coal Basin in Poland-were investigated. The coal samples contained variable amounts of siderite, dolomite, calcite, kaolinite, illite, quartz, apatite, and pyrite in their mineral composition. A five-step sequential chemical leaching procedure was used, including deionized water, 3% HCl, 5% HNO(3), 10% HNO(3) with microwave assistance, and concentrated HCl-HF also with microwave assistance. The highest concentrations of ∑REY were observed in seam 404/1. Light REY (LREY) dominated the REY composition (>75%), while heavy REY (HREY) accounted for less than 10%. The chondrite-normalised REY patterns and total REY content indicate a clastic origin of REY-bearing minerals. The most efficient leaching occurred in stages IV and V. The solutions from stages I-III preferentially mobilised critical REY, while those from stages IV-V reflected the REY distribution in the coal. Based on the C(outl) index, both coal and leachates from the later stages are classified as prospective REY resources. However, absolute REY concentrations should be considered when interpreting C(outl) values. The positive correlation between apatite and kaolinite contents and ∑REE concentrations suggests their role in REY enrichment.

特别声明

1、本页面内容包含部分的内容是基于公开信息的合理引用;引用内容仅为补充信息,不代表本站立场。

2、若认为本页面引用内容涉及侵权,请及时与本站联系,我们将第一时间处理。

3、其他媒体/个人如需使用本页面原创内容,需注明“来源:[生知库]”并获得授权;使用引用内容的,需自行联系原作者获得许可。

4、投稿及合作请联系:info@biocloudy.com。