An improved synthesis of telmisartan via the copper-catalyzed cyclization of o-haloarylamidines

通过铜催化邻卤代芳基脒环化反应改进替米沙坦的合成

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Abstract

A concise synthetic route was designed for making telmisartan. The key bis-benzimidazole structure was constructed via the copper-catalyzed cyclization of o-haloarylamidines. By adopting this approach, telmisartan was obtained in a 7-step overall yield of 54% starting from commercially available 3-methyl-4-nitrobenzoic acid, and the use of HNO(3)/H(2)SO(4) for nitration and polyphosphoric acid (PPA) for cyclization in the reported literatures were avoided.

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