Hydrogen Sulfide Mediated Tandem Reaction of Selenenyl Sulfides and Its Application in Fluorescent Probe Development

硫化氢介导的硒代硫醚串联反应及其在荧光探针开发中的应用

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Abstract

A unique reaction between H(2)S and a selenenyl sulfide containing benzoate ester template was discovered. This reaction could be specifically triggered by H(2)S and lead to ester bond cleavage. The reaction was not affected by the presence of thiols such as glutathione and cysteine. With this reaction, a series of fluorescent probes were synthesized and evaluated. The probes exhibited high sensitivity/selectivity for H(2)S in both buffers and cells.

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