Research on the Formation Conditions and Preventive Measures of Uranium Precipitates during the Service Process of Medical Isotope Production Reactors

医用同位素生产反应堆服役过程中铀沉淀形成条件及预防措施研究

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作者:Yanli Zhao, Yuan Gao, Xinyue Li, Yi Le, Yang Zhang, Jie Qiu, Yong Xin

Abstract

This study focuses on the Medical Isotope Production Reactor (MIPR), an aqueous homogeneous reactor utilized for synthesizing medical isotopes like 99Mo. A pivotal aspect of MIPR's functionality involves the fuel solution's complex chemical interactions, particularly during reactor operation. These interactions result in the formation of precipitates, notably water filamentous uranium ore and columnar uranium ore, which can impact reactor performance. The research presented here delves into the reactions between liquid fuel uranyl nitrate and key radiolytic products, employing simulation calculations complemented by experimental validation. This approach facilitates the identification of uranium precipitate types and their formation conditions under operational reactor settings. Additionally, the article explores strategies to mitigate the formation of specific uranium precipitates, thereby contributing to the efficient and stable operation of MIPR.

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