Synthesis of a highly stable Mo-Fe bimetallic metal-organic framework and its catalytic activity for the selective oxidation of sulfides under mild conditions

合成了一种高稳定性钼铁双金属有机框架化合物及其在温和条件下选择性氧化硫化物的催化活性

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Abstract

A novel Mo-Fe bimetallic metal-organic framework [Fe(2)(4,4'-bipy)Mo(2)O(8)]·2H(2)O (1) was synthesized and characterized by X-ray single crystal diffraction, infrared spectroscopy (IR), thermogravimetric analysis (TGA), ultraviolet-visible spectroscopy (UV-vis), and its magnetic properties were studied. The compound demonstrates insolubility in most solvents and exhibits significant chemical stability across a wide pH range. Typically, exceptional selectivity and efficient conversion of sulfides to sulfoxides using 1 with H(2)O(2) have been verified under ambient conditions.

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