Palladium-Catalyzed α-Arylation of Methyl Sulfonamides with Aryl Chlorides

钯催化甲基磺酰胺与芳基氯化物的α-芳基化反应

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Abstract

A Palladium-catalyzed α-arylation of sulfonamides with aryl chlorides is presented. A Buchwald type precatalyst formed with Kwong's indole-based ligand enabled this transformation to be compatible with a large variety of methyl sulfonamides and aryl chlorides in good to excellent yields. Importantly, under the optimized reaction conditions, only mono-arylated products were observed. This method has been applied to the efficient synthesis of sumatriptan, which is used to treat migraines.

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