Enantioselective synthesis of metacycloprodigiosin via the "Wasserman pyrrole"

通过“瓦瑟曼吡咯”实现间环丙二红素的对映选择性合成

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Abstract

A concise, nine-step enantioselective total synthesis of metacycloprodigiosin is reported. The synthesis provides increased step-efficiency over the previous racemic and enantioselective syntheses of this compound. Key features of the work include investigations into a convergent oxidative coupling reaction and subsequent ring-closing metathesis to deliver an advanced pyrrole intermediate we name the "Wasserman pyrrole" that can be converted to metacycloprodigiosin in one step.

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