Solvent-controlled self-assembly of tetrapodal [4 + 4] phosphate organic molecular cage

溶剂控制的四足[4+4]磷酸有机分子笼的自组装

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Abstract

Two flexible subcomponents, namely tris(4-formylphenyl)phosphate and tris(2-aminoethyl)amine, are assembled into a tetrapodal [4 + 4] cage depending on the solvent effect. Single-crystal structure analysis reveals that the caivity is surrounded by four phosphate uints. Good selectivity of CO(2) adsorption over CH(4) is demonstrated by the gas adsorption experiment.

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