Investigating metal (M = Mn, Fe, and Ni)-doped Co(OH)(2) nanofibers for electrocatalytic oxygen evolution and electrochemical biosensing performance

研究金属(M = Mn、Fe 和 Ni)掺杂的 Co(OH)₂ 纳米纤维的电催化析氧性能和电化学生物传感性能

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Abstract

To achieve efficient and cost-effective electrochemical water splitting, highly active and affordable nanostructured catalysts are the key requirement. The current study presents the investigations of the efficacy of metal (Mn, Fe and Ni)-doped Co(OH)(2) nanofibers towards oxygen evolution via water splitting. Notably, Ni-doped Co(OH)(2) demonstrates superior OER performance in KOH electrolyte, surpassing standard IrO(2) with a modest potential of 1.62 V at 10 mA cm(-2). The remarkable activity is attributed to the nanofiber structure, facilitating faster conduction and offering readily available active sites. Ni-doped Co(OH)(2) nanofibers displayed enduring stability even after 1000 cycles. This work underscores the importance of transition-metal based catalysts as effective electrocatalysts, providing the groundwork for the development of cutting-edge catalysts. Additionally, the electrochemical sensing capability towards ascorbic acid is evaluated, with Ni-doped Co(OH)(2) showing the most promising response, characterized by the lowest LOD and LOQ values. These findings highlight the potential of Ni-doped Co(OH)(2) nanofibers for upcoming diagnostic detection devices.

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