Conversion of Phenol and Lignin as Components of Renewable Raw Materials on Pt and Ru-Supported Catalysts

以Pt和Ru为载体的催化剂转化苯酚和木质素等可再生原料组分

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Abstract

Hydrogenation of phenol in aqueous solutions on Pt-Ni/SiO(2), Pt-Ni-Cr/Al(2)O(3), Pt/C, and Ru/C catalysts was studied at temperatures of 150-250 °C and pressures of 40-80 bar. The possibility of hydrogenation of hydrolysis lignin in an aqueous medium in the presence of a Ru/C catalyst is shown. The conversion of hydrolysis lignin and water-soluble sodium lignosulfonate occurs with the formation of a complex mixture of monomeric products: a number of phenols, products of their catalytic hydrogenation (cyclohexanol and cyclohexanone), and hydrogenolysis products (cyclic and aliphatic C(2)-C(7) hydrocarbons).

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