Asymmetric Induction by a Nitrogen (14) N/(15) N Isotopomer in Conjunction with Asymmetric Autocatalysis

氮(14)N/(15)N同位素异构体与不对称自催化的不对称诱导

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Abstract

Chirality arising from isotope substitution, especially with atoms heavier than the hydrogen isotopes, is usually not considered a source of chirality in a chemical reaction. An N(2) ,N(2) ,N(3) ,N(3) -tetramethyl-2,3-butanediamine containing nitrogen ((14) N/(15) N) isotope chirality was synthesized and it was revealed that this isotopically chiral diamine compound acts as a chiral initiator for asymmetric autocatalysis.

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