Synthesis of Ion-Exchange Catalysts by Introduction of Fluorinated Ponytails into Novel Mesoporous Polymers

通过将氟化尾链引入新型介孔聚合物中合成离子交换催化剂

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Abstract

A novel synthetic procedure for the functionalisation of styrenic cross-linked polymers with perfluorinated acyl chains has been reported. The effective significant grafting of the fluorinated moieties is supported by {(1)H}-(13)C and {(19)F}-(13)C NMR characterisations. This kind of polymer appears promising as catalytic support for a variety of reactions requiring a highly lipophilic catalyst. Indeed, the improved lipophilicity of the materials resulted in enhanced catalytic properties of the corresponding sulfonic materials in the reaction of esterification of a solution in a vegetable oil of stearic acid with methanol.

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