Abstract
Two-dimensional (2D) magnetic materials exhibiting unique 2D-limit magnetism have attracted great attention due to their potential applications in ultrathin spintronic devices. These 2D magnetic materials and their heterostructures provide a unique platform for exploring physical effect and exotic phenomena. However, the degradation of most 2D magnetic materials at ambient conditions has so far hindered their characterization and integration into ultrathin devices. Furthermore, the effect of degradation on magnetoelectric transport properties, which is measured for the demonstration of exotic phenomena and device performance, has remained unexplored. Here, the first experimental investigation of the degradation of CrBr(3) flakes and its effect on magnetoelectric transport behavior in devices is reported. The extra magnetic compounds derived from oxidation-related degradation play a significant role in the magnetoelectric transport in CrBr(3) devices, greatly affecting the magnetoresistance and conductivity. This work has important implications for studies concerning 2D magnetic materials measured, stored, and integrated into devices at ambient conditions.