Microwave assisted green synthesis of Fe(2)O(3)/biochar for ultrasonic removal of nonsteroidal anti-inflammatory pharmaceuticals

微波辅助绿色合成Fe(2)O(3)/生物炭用于超声去除非甾体抗炎药物

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Abstract

Iron oxide/biochar (Fe(2)O(3)/biochar) was prepared by green synthesis via a microwave to evaluate ultrasound-assisted adsorption capacity of Nonsteroidal Anti-inflammatory Drugs (NSAIDs) (salicylic acid, naproxen, and ketoprofen) from the water. Several techniques of characterization, including, Fourier transform infrared spectrometry, scanning electron microscopy, EDS analysis, N(2) adsorption-desorption, X-ray diffraction, and Raman spectrometry were applied. The adsorption of NSAIDs onto Fe(2)O(3)/biochar was performed using an ultrasonic bath. The effects of batch adsorption under various experimental parameters such as contact time (0-120 min), initial concentration (10-500 mg L(-1)) and pH (2-12) were tested. The obtained Fe(2)O(3)/biochar specific surface area, mesopore volume/micropore volume, and pores size were equal to 786 m(2) g(-1), 0.409 cm(3) g(-1), and 1.534 cm(3) g(-1), respectively. The pseudo-second-order model could describe better all NSAID adsorptions onto Fe(2)O(3)/biochar. The Langmuir model agreed well with the NSAID adsorptions and the maximum adsorption capacities reached 683 mg g(-1), 533 mg g(-1) and 444 mg g(-1) for salicylic acid, naproxen, and ketoprofen, respectively. Fe(2)O(3)/biochar can be used as an excellent adsorbent for the treatment of NSAIDs in water.

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