Palladium catalyst imbedded in polymers of intrinsic microporosity for the Suzuki-Miyaura coupling reaction

用于 Suzuki-Miyaura 偶联反应的嵌入具有固有微孔性的聚合物中的钯催化剂

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Abstract

Polymers of intrinsic microporosity (PIMs) are porous polymers with rigid ladder-type chain structures. Synthesizing these polymers usually involves the step polymerization of two types of monomer, namely, active fluorine-substituted aromatic ring monomers and phenolic monomers. Herein, we report a new PIMs preparation method using self-synthesized fluorinated monomers and common monomer 5,5',6,6'-tetrahydroxy-3,3,3',3'-tetramethyl spirobisindane. The fluorinated monomers were synthesized through the imidization of tetrafluorophthalic anhydride and aromatic diamines. The resulting PIMs served as a support for palladium, with the formed catalyst showing potential for application in the Suzuki-Miyaura coupling reaction.

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