A Comparative Study on the Addition Methods of TiO₂ Sintering Aid to the Properties of Porous Alumina Membrane Support

二氧化钛烧结助剂添加方法对多孔氧化铝膜支撑体性能的影响比较研究

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Abstract

TiO₂ is usually used as a sintering aid to lower the sintering temperature of porous alumina membrane support. Two ways of the addition of TiO₂ are chosen: in-situ precipitation and in-situ hydrolysis. The results show that the distribution status of TiO₂ has an important effect on the property of porous alumina membrane support. In in-situ hydrolysis method, the nano-meter scale TiO₂ distributes evenly on the alumina particles' surface. The bending strength of the support increases sharply and the pore size distribution changes more sharply along with the content of TiO₂ which slightly increases from 0.3 wt.% to 0.4 wt.%. The distribution of the nano-meter scale TiO₂ is not so even added by in-situ precipitation method. Neither the bending strength nor the pore size distribution of the support is worse than that of the support added by in-situ hydrolysis even if the content of TiO₂ is high to 2 wt.%. The permeating flux has a similar tendency. Consequently, the porous alumina membrane support has the porosity of 30.01% and the bending strength of 77.33 MPa after sintering at 1650 °C for 2 h with the optimized TiO₂ content of 0.4 wt.% added by the in-situ hydrolysis method.

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