Hierarchical nickel carbonate hydroxide nanostructures for photocatalytic hydrogen evolution from water splitting

用于光催化分解水制氢的分级镍碳酸氢氧化物纳米结构

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Abstract

Metal carbonate hydroxides have emerged as novel and promising candidates for water splitting due to their good electrochemical properties and eco-friendly features. In this study, the hierarchical mesoporous structure of nickel carbonate hydroxide hydrate (Ni(2)(CO(3))(OH)(2)·4H(2)O) was synthesized by a one-pot facile hydrothermal method. It demonstrated photocatalytic properties for the first time, exhibiting a hydrogen evolution reaction yield of 10 μmol g(-1) h(-1) under white light irradiation with a nominal power of 0.495 W. This facile synthesis strategy and the good photocatalytic properties indicate that nickel carbonate hydroxide is a promising material for application in photocatalytic hydrogen evolution.

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