Eco-efficient symbio-pozzolanic hydrophobic cementitious binders for sustainable and durable infrastructure

用于可持续和耐久基础设施的生态高效共生火山灰疏水性水泥粘合剂

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Abstract

This study presents the development of an internally hydrophobic cementitious binder through the incorporation of a Symbio-Pozzolanic Composite Hydrophobic Powder (SPCHP), synthesized from fly ash, silica fume, metakaolin, and zinc stearate. SPCHP was introduced as a partial cement replacement at levels ranging from 5% to 40%, and its effects were systematically evaluated in terms of fresh properties, mechanical performance, durability, microstructural behaviour, and cost efficiency. The mix containing 25 wt% SPCHP (HP25) exhibited the most balanced performance, achieving 73% of the compressive strength of the control mortar while imparting strong hydrophobicity (water contact angle of 114°) and reducing water absorption to 4.2%. Enhanced resistance against chloride ingress, sulphate and acid attack, along with improved ultrasonic pulse velocity, confirmed the role of SPCHP in densifying the microstructure and reducing transport properties. Life-cycle benefits were demonstrated through lower CO₂ emissions and favourable cost-to-strength ratios. These findings establish SPCHP as a sustainable material innovation for prolonging the service life of cement-based structures in aggressive environments, with potential for scalable engineering applications.

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