Abstract
As the only natural source of aromatic biopolymers, lignin can be converted into value-added chemicals and biofuels, showing great potential in realizing the development of green chemistry. At present, lignin is predominantly used for combustion to generate energy, and the real value of lignin is difficult to maximize. Accordingly, the depolymerization of lignin is of great significance for its high-value utilization. This review discusses the latest progress in the field of lignin depolymerization, including catalytic conversion systems using various thermochemical, chemocatalytic, photocatalytic, electrocatalytic, and biological depolymerization methods, as well as the involved reaction mechanisms and obtained products of various protocols, focusing on green and efficient lignin depolymerization strategies. In addition, the challenges faced by lignin depolymerization are also expounded, putting forward possible directions of developing lignin depolymerization strategies in the future.