Magnetic Biochar Derived from Waste Bamboo as a Peroxymonosulfate Activator for Tetracycline Hydrochloride Degradation

以废弃竹子为原料制备的磁性生物炭作为过一硫酸盐活化剂用于四环素盐酸盐降解

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Abstract

Magnetic Fe and N-doped biochar (FeN-BC) was synthesized from waste bamboo through microwave pyrolysis and used as a catalyst for the degradation of tetracycline hydrochloride (TC) with peroxymonosulfate (PMS). The results showed that doping with Fe improved the recovery performance of biochar and the N-doping enhanced the activity of PMS. Simultaneously, it achieved a high degradation efficiency for TC (93%) under optimized conditions within 30 min. Electron paramagnetic resonance (EPR) and quenching experiments indicated that the main active radicals present in the experiment were SO(4)(•-) and •OH. Additionally, FeN-BC demonstrated good catalytic performance in the TC degradation process in a real water environment after five cycles. This work presents a practical strategy for preparing magnetic biochar to degrade organic pollutants from wastewater.

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