Single-Base Detection of DNA with Simplified Steps on InGaN Quantum Wells

基于InGaN量子阱的简化步骤DNA单碱基检测

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Abstract

DNA testing is a powerful tool to evaluate an individual's risk for genetic disorders or certain illnesses. Completing the test quickly and accurately is the key to preventing many deadly diseases. However, the work is usually a tedious process as it entails multiple steps of molecular modification. To address the challenge, we present a simplified DNA detection tactic, skipping surface functionalization, fluorescent labeling, and probe immobilization. In addition, we show that a wide-field (9 × 9 μm(2)) submicron image of dilute DNA (1 × 10(-9) M) can be captured in a 3.5 min single laser exposure. The task is accomplished by surface-enhanced Raman spectroscopy (SERS) built with InGaN quantum wells covered by Al nanospheres. This unique biochip makes the nucleotide fully exposed to the SERS hot surface, catching the single-base DNA signal with single-molecule sensitivity.

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