Nanopatterning of Perovskite Thin Films for Enhanced and Directional Light Emission

钙钛矿薄膜的纳米图案化可增强定向光发射

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作者:Loreta A Muscarella, Andrea Cordaro, Georg Krause, Debapriya Pal, Gianluca Grimaldi, Leo Sahaya Daphne Antony, David Langhorst, Adrian Callies, Benedikt Bläsi, Oliver Höhn, A Femius Koenderink, Albert Polman, Bruno Ehrler

Abstract

Lead-halide perovskites offer excellent properties for lighting and display applications. Nanopatterning perovskite films could enable perovskite-based devices with designer properties, increasing their performance and adding novel functionalities. We demonstrate the potential of nanopatterning for achieving light emission of a perovskite film into a specific angular range by introducing periodic sol-gel structures between the injection and emissive layer by using substrate conformal imprint lithography (SCIL). Structural and optical characterization reveals that the emission is funnelled into a well-defined angular range by optical resonances, while the emission wavelength and the structural properties of the perovskite film are preserved. The results demonstrate a flexible and scalable approach to the patterning of perovskite layers, paving the way toward perovskite LEDs with designer angular emission patterns.

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