Polyaniline-functionalized Nb(2)CT(x) Mxene composites for effective Cr(VI) adsorption from wastewater

聚苯胺功能化的Nb(2)CT(x)MXene复合材料可有效吸附废水中的Cr(VI)

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Abstract

In this study Nb(2)CT(x)/PANI nanocomposite was reported for the adsorption of Cr(VI) from contaminated water samples for the first time. The unique structure of Nb(2)CT(x) Mxene, combined with the conductive and adsorptive properties of polyaniline (PANI), forms a high-surface-area composite with enhanced affinity for Cr(VI) ions. The synthesized nanocomposite was characterized by using different techniques XRD, FTIR, BET, SEM-EDX, XPS and Raman spectroscopy. Influence of various parameters such as pH, dosage, and initial ion concentration on adsorption were also studied. Adsorption experiments demonstrate that Nb(2)CT(x)/PANI exhibits a high adsorption capacity, achieving a maximum Cr(VI)removal efficiency of 468.35 mg/g. Freundlich model is used to describe the experimental data of the adsorption system, where the calculated values of q(max) agree with the experimental data, with a reasonable determination coefficient (R(2) = 0.876). The Nb(2)CT(x)/PANI MXene showed effective adsorption of Cr(VI)ions via multilayer adsorption, the mechanism involves electrostatic attraction, ion exchange, hydrogen bonding, surface complexation, and reduction. This study highlights the synergistic effect of Nb(2)CT(x) Mxene and PANI in developing high-performance adsorbents for heavy metal removal, offering a promising approach for environmental remediation.

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