Crystal structure, Hirshfeld surface analysis and DFT study of (2Z)-2-(2,4-di-chloro-benzyl-idene)-4-[2-(2-oxo-1,3-oxazolidin-3-yl)eth-yl]-3,4-di-hydro-2H-1,4-benzo-thia-zin-3-one

(2Z)-2-(2,4-二氯苄基亚甲基)-4-[2-(2-氧代-1,3-噁唑烷-3-基)乙基]-3,4-二氢-2H-1,4-苯并噻嗪-3-酮的晶体结构、Hirshfeld表面分析和DFT研究

阅读:1

Abstract

The title compound, C(20)H(16)Cl(2)N(2)O(3)S, is built up from a di-hydro-benzo-thia-zine moiety linked by -CH- and -C(2)H(4)- units to 2,4-di-chloro-phenyl and 2-oxo-1,3-oxazolidine substituents, where the oxazole ring and the heterocyclic portion of the di-hydro-benzo-thia-zine unit adopt envelope and flattened-boat conformations, respectively. The 2-carbon link to the oxazole ring is nearly perpendicular to the mean plane of the di-hydro-benzo-thia-zine unit. In the crystal, the mol-ecules form stacks extending along the normal to (104) with the aromatic rings from neighbouring stacks inter-calating to form an overall layer structure. The Hirshfeld surface analysis of the crystal structure indicates that the most important contributions for the crystal packing are from H⋯H (28.4%), H⋯Cl/Cl⋯H (19.3%), H⋯O/O⋯H (17.0%), H⋯C/C⋯H (14.5%) and C⋯C (8.2%) inter-actions. Weak hydrogen-bonding and van der Waals inter-actions are the dominant inter-actions in the crystal packing. Density functional theory (DFT) optimized structures at the B3LYP/ 6-311 G(d,p) level are compared with the experimentally determined mol-ecular structure in the solid state. The HOMO-LUMO behaviour was elucidated to determine the energy gap.

特别声明

1、本页面内容包含部分的内容是基于公开信息的合理引用;引用内容仅为补充信息,不代表本站立场。

2、若认为本页面引用内容涉及侵权,请及时与本站联系,我们将第一时间处理。

3、其他媒体/个人如需使用本页面原创内容,需注明“来源:[生知库]”并获得授权;使用引用内容的,需自行联系原作者获得许可。

4、投稿及合作请联系:info@biocloudy.com。