Bacterial Cellulose-Based Laser-Scribed Graphene Electrode for Hydrogen Peroxide Detection in Cancer Cells

基于细菌纤维素的激光刻蚀石墨烯电极用于癌细胞中过氧化氢的检测

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Abstract

The development of sustainable and high-performance electrochemical sensors is crucial for advancing biomedical applications. In this work, we introduce a hydrogen peroxide (H(2)O(2)) sensor based on bacterial cellulose-derived laser-scribed graphene (BC-LSG), modified with MXene and platinum nanoparticles (PtNPs). Bacterial cellulose (BC), a biodegradable and renewable material, was cultivated and transformed into a highly conductive carbon network using CO(2) laser irradiation, producing a flexible, portable, and miniaturized electrochemical platform. The incorporation of MXene and PtNPs significantly enhanced the electrocatalytic response toward H(2)O(2) oxidation, achieving a wide linear concentration range (15-95 μmol L(-1)) and a low detection limit (0.35 μmol L(-1)). Compared to traditional enzymatic sensors, our nanostructured BC-LSG device offers superior stability, reproducibility, and eco-friendliness, aligning with green analytical chemistry principles. The sensor was successfully applied for H(2)O(2) detection in mammalian cells, demonstrating its potential for real-time monitoring of oxidative stress, a key biomarker in cancer progression and therapeutic responses. This work underscores the synergy between biopolymeric materials, nanotechnology, and laser processing, opening new avenues for scalable, disposable, and sustainable electrochemical devices.

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