Identifying key molecular interactions and pathways linking DEHP and its metabolite MEHP to allergic rhinitis: a network toxicology and molecular dynamics study

识别邻苯二甲酸二(2-乙基己基)酯(DEHP)及其代谢物邻苯二甲酸二(2-乙基己基)酯(MEHP)与过敏性鼻炎相关的关键分子相互作用和通路:一项网络毒理学和分子动力学研究

阅读:1

Abstract

BACKGROUND: Di-(2-ethylhexyl) phthalate (DEHP) and its major metabolite mono-(2-ethylhexyl) phthalate (MEHP) are ubiquitous environmental contaminants increasingly implicated in allergic rhinitis (AR). However, their molecular mechanisms remain unclear. This study aimed to employ a computational toxicology approach to predict DEHP/MEHP-associated toxicological targets and pathways relevant to AR and to screen for key mediators underpinning this association. METHODS: Putative targets of DEHP and MEHP were compiled using SEA, SwissTargetPrediction, and TargetNet, while AR-related genes were curated from GeneCards, DrugBank, OMIM, DisGeNET, and PharmGKB. After deduplication, overlapping targets were analyzed via STRING-based protein–protein interaction (PPI) networks and GO/KEGG enrichment. Specifically, unique targets common to DEHP, MEHP, and AR were identified and prioritized. Expression of the core target was evaluated in the GSE52804 dataset (OVA-induced AR mouse model). Molecular docking assessed binding of DEHP/MEHP to PTGS2, followed by molecular dynamics (MD) simulations and free energy landscape (FEL) analyses. RESULTS: We identified 370 unique predicted targets of DEHP/MEHP and 1,213 genes associated with AR, yielding 71 overlapping genes. Functional enrichment analysis of these overlaps suggested their potential involvement in inflammatory and immune pathways. Among these, 21 targets common to DEHP, MEHP, and AR were predicted to be associated with key biological processes such as cellular response to environmental stimulus. PPI network topology analysis indicated PTGS2 as a central hub gene. Molecular docking predicted moderate affinity for both ligands, with scores of − 6.4 for DEHP and − 7.6 for MEHP to PTGS2. MD simulations demonstrated the stability of both predicted complexes, with consistent binding free energies and the presence of persistent hydrogen bonds. FELs showed well-defined global minima for both complexes. CONCLUSIONS: This in silico analysis predicts potential multi-target interactions between DEHP/MEHP and proteins implicated in AR pathogenesis. Among these, PTGS2 emerged as a high-priority candidate based on network topology and molecular docking evaluations. The computational results identify PTGS2 and other hub targets as candidates for experimental validation in the context of DEHP/MEHP exposure. SUPPLEMENTARY INFORMATION: The online version contains supplementary material available at 10.1186/s40360-026-01098-z.

特别声明

1、本页面内容包含部分的内容是基于公开信息的合理引用;引用内容仅为补充信息,不代表本站立场。

2、若认为本页面引用内容涉及侵权,请及时与本站联系,我们将第一时间处理。

3、其他媒体/个人如需使用本页面原创内容,需注明“来源:[生知库]”并获得授权;使用引用内容的,需自行联系原作者获得许可。

4、投稿及合作请联系:info@biocloudy.com。