Electron and spin dynamics in a single quantum emitter

单个量子发射器中的电子和自旋动力学

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Abstract

The Auger-Meitner effect is a fundamental electron-electron scattering process that impacts the electron and spin dynamics in semiconductor quantum emitters, such as colloidal nanocrystals and quantum dots. Here, we present an experimental study of the magnetic-field dependence of Auger-Meitner recombination and spin-related scattering processes in a single self-assembled InAs quantum dot. Using two-color, time-resolved resonance fluorescence with spectrally separated detection of both exciton and trion transitions, we extract the Auger-Meitner recombination rate, the electron spin-flip relaxation rate, and the spin-flip Raman scattering rate over a broad magnetic-field range from B = 0 to 8 T . We observe a suppression of the Auger-Meitner recombination rate for magnetic fields above B = 4 T . In contrast, the electron spin-flip relaxation rate increases strongly for fields above B = 3 T and decreases at lower magnetic fields, while the spin-flip Raman scattering rate remains nearly constant. Our results demonstrate that two-color, time-resolved resonance fluorescence enables access to all relevant microscopic rates for optimizing quantum dots as building blocks for future quantum technologies.

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