DFT study of frontier orbitals and NLO properties of a phenanthroline and nitrophenol complex

利用密度泛函理论(DFT)研究菲咯啉和硝基苯酚复合物的前线轨道和非线性光学性质

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Abstract

The hydrogen-bond charge transfer complex (HB-CTC) formed between the donor, 1,10-phenanthroline (Phen), and the π-acceptor, p-nitrophenol (PNP), has been thoroughly investigated through theoretical studies. The molecular structure and the HOMO-LUMO energy gap (ΔE(H-L)) of this complex have been investigated by the density functional theory. This work has studied the HB-CTC complex through FTIR, (1)HNMR, (13)CNMR, and electronic absorption spectra. A molecular electrostatic potential surface (MESP) study allowed us to explore key aspects of intermolecular interaction. Moreover, reduced density gradient analysis was conducted to visualize valuable insights into non-covalent interactions within the complex components. Quantum Theory of Atoms in Molecules was used to analyze the interaction between the 1,10-phenanthroline and p-nitrophenol. The findings from this research not only enhance our understanding of HB-CT complexes but also highlight their exciting potential for innovative applications in various fields.

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