Distinct Responses of Corrosion Behavior to the Intermetallic/Impurity Redistribution During Hot Processing in Micro-Alloyed Mg Alloys

微合金化镁合金热加工过程中金属间化合物/杂质重新分布对腐蚀行为的不同影响

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Abstract

By tuning the extrusion parameters, the corrosion performances of as-extruded Mg-0.5Zn(-0.2X) alloys (X: Ca/Sr/Ag/In/Cu, denoted as Z05, Z0502-Ca, Z0502-Sr, Z0502-Ag, Z0502-In and Z0502-Cu, respectively) with similar grain sizes were investigated and compared with their as-cast counterparts. The formed Fe-Si precipitates after hot processing significantly accelerate the corrosion rates of Z05, Z0502-Ag and Z0502-In, whereas the driving force from the Fe-encapsulated MgCaSi(Fe) and MgSrSi(Fe) precipitates are not as strong in Z0502-Ca and Z0502-Sr. Impacts from Fe impurity in Z0502-Cu are masked in the fast corrosion due to the noble Mg2Cu intermetallics. Fe precipitation during hot processing is critical for micro-alloyed systems, as the changes in intermetallic/impurity distributions impact the corrosion performances profoundly. The enthalpy of formation and the potential difference are the key factors that influence the distribution of precipitate during hot processing.

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