Direct observation of the collective modes of the charge density wave in the kagome metal CsV3Sb5

直接观察 kagome 金属 CsV3Sb5 中的电荷密度波的集体模式

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作者:Doron Azoury #, Alexander von Hoegen #, Yifan Su, Kyoung Hun Oh, Tobias Holder, Hengxin Tan, Brenden R Ortiz, Andrea Capa Salinas, Stephen D Wilson, Binghai Yan, Nuh Gedik

Abstract

A recently discovered group of kagome metals AV[Formula: see text]Sb[Formula: see text] (A = K, Rb, Cs) exhibit a variety of intertwined unconventional electronic phases, which emerge from a puzzling charge density wave phase. Understanding of this charge-ordered parent phase is crucial for deciphering the entire phase diagram. However, the mechanism of the charge density wave is still controversial, and its primary source of fluctuations-the collective modes-has not been experimentally observed. Here, we use ultrashort laser pulses to melt the charge order in CsV[Formula: see text]Sb[Formula: see text] and record the resulting dynamics using femtosecond angle-resolved photoemission. We resolve the melting time of the charge order and directly observe its amplitude mode, imposing a fundamental limit for the fastest possible lattice rearrangement time. These observations together with ab initio calculations provide clear evidence for a structural rather than electronic mechanism of the charge density wave. Our findings pave the way for a better understanding of the unconventional phases hosted on the kagome lattice.

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