Abstract
Spatially resolved measurements of the argon excimer, Ar2 ∗ , were performed in the effluent of a cold atmospheric plasma jet (CAPJ), the so called kINPen-sci, using cavity ringdown spectroscopy. The spatial distribution of the density of Ar2 ∗ could be distinguished into two distinct populations: a Gaussian and a toroidally shaped distribution. The production mechanisms of these populations seem to differ. On the one hand, a strong correlation was found between the Gaussian Ar2 ∗ population and the spatial distribution of the filaments produced in the effluent of the kINPen-sci. On the other hand, measurements performed while varying the experimental conditions under which the kINPen-sci was operated indicate that the gas flow velocity must play a major role in the formation of the toroidal Ar2 ∗ population. However, the mechanism of formation of the toroid Ar2 ∗ population remains unclear.