Quantum-mechanical equilibrium isotopic fractionation correction to radiocarbon dating: a theory study

量子力学平衡同位素分馏校正在放射性碳定年中的应用:理论研究

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Abstract

This paper relates the quantum-mechanical equilibrium isotopic fractionation correction to the radiocarbon dating method by Eq. 9, and also shows the significant influence of temperature on the method. It is suggested that the correction is a function of the frequencies and temperature of a specific sample and these two variables can be evaluated theoretically by the ab initio quantum calculations and experimentally by analyzing the clumped-isotope ratios in it, respectively. This paper also suggests that the (14)C/(12)C ratio in the atmosphere in geological time can be calculated by Eq. 10.

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