Structure, Intrinsic properties and Vibrational Spectra of Pr(Mg(1/2)Sn(1/2))O(3) Ceramic Crystal

Pr(Mg<sub>1/2</sub>Sn<sub>1/2</sub>)O<sub>3</sub>陶瓷晶体的结构、本征性质和振动光谱

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Abstract

Pr(Mg(1/2)Sn(1/2))O(3) (PMS) ceramic was prepared through a conventional solid-state reaction method. Crystal structure was investigated through X-ray diffraction (XRD), which certificates that the main phase is PMS with monoclinic P2 (1)/n1 symmetry. Lattice vibrational modes were obtained through Raman scattering spectroscopy and Fourier transform far-infrared reflection spectroscopy. The Raman spectrum active modes were assigned and illustrated, respectively, and then fitted with Lorentzian function. The four modes within the range of 110-200 cm(-1) are derived from the F (2g) vibrations (A-site cations), and the other three modes (300-430 cm(-1)) are derived from the F (2g) vibrations (B-site cations).The mode with highest frequency above 650 cm(-1) is attributed to A (1g) -like mode that corresponds to the symmetric breathing of oxygen octahedral. The far-infrared spectrum with seven infrared active modes was fitted using four-parameter semi-quantum models to calculate intrinsic properties (permittivity and loss). F (2u)((2)) yielded the greatest contribution to dielectric constant and loss, which is mainly performed as the inverted translational vibration of Pr-MgO(6) octahedron.

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