The Impact of Cyclic Oxidation in Dissociated Air on the Mechanical Properties of Freeze-Cast ZrB(2)/MoSi(2) Ceramics

循环氧化在分解空气中对冷冻铸造ZrB(2)/MoSi(2)陶瓷力学性能的影响

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Abstract

Creating reusable thermal shields would decrease our carbon footprint by eliminating the need for the reapplication of single-use ablative alternatives. Our previous investigations identified ultra-high-temperature ZrB(2) with 20 vol.% MoSi(2) ceramics as a promising candidate for the fabrication of reusable thermal shields. Therefore, in this study, this material was exposed to cyclic oxidation at 1800 and 2150 K in dissociated air in order to investigate how it might withstand multiple terrestrial re-entries. At 1800 K, we observed semi-parabolic oxidation kinetics with the growth of a protective oxide layer, the silica-based composition of which was determined using XRD and SEM (coupled with EDS). More dramatic damage was observed at 2150 K, with continuous linear oxidation kinetics seen. Cross-section hardness measurements using nanoindentation revealed that the oxidized part of the samples was the source of their mechanical weakness, suggesting that the material should be used below 1800 K to ensure its reusability.

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