Enhancing Plant Fibre-Reinforced Polymer Composites for Biomedical Applications Using Atmospheric Pressure Plasma Treatment

利用大气压等离子体处理增强植物纤维增强聚合物复合材料在生物医学应用中的性能

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Abstract

This research investigates the effects of corona plasma treatment on the mechanical properties of jute/epoxy-reinforced composites, particularly within biomedical application contexts. Plant Fibre Composites (PFCs) are attractive for medical devices and scaffolds due to their environmental friendliness, renewability, cost-effectiveness, low density, and high specific strength. However, their applications are often constrained by inferior mechanical performance arising from poor bonding between the plant fibre used as the reinforcement and the synthetic resin or polymer serving as the matrix. This study addresses the challenge of improving the weak interfacial bonding between plant fibre and synthetic resin in a 2/2 twill-weave-woven jute/epoxy composite material. The surface of the jute fibre is modified for better adhesion with the epoxy resin through plasma treatment, which exposes the jute fibre to controlled plasma energy and utilises dry air (plasma only), argon (Ar) (argon gas with plasma), and nitrogen (N(2)) (nitrogen gas with plasma) at two different distances (25 mm and 35 mm) between the plasma nozzle and the fibre surface. In this context, "equilibrium" refers to the optimal combination of plasma power, treatment distance, and gas environment that collectively determines the degree of fibre surface modification. The results indicate that all plasma treatments improve the interlaminar shear strength in comparison to untreated samples, with treatments at 35 mm using N(2) gas showing a 35.4% increase in shear strength. Conversely, plasma treatment using dry air at 25 mm yields an 18.3% increase in tensile strength and a 35.7% increase in Young's modulus. These findings highlight the importance of achieving an appropriate equilibrium among plasma intensity, treatment distance, and fibre-plasma interaction conditions to maximise the effectiveness of plasma treatment for jute/epoxy composites. This research advances sustainable innovation in biomedical materials, underscoring the potential for improved mechanical properties in environmentally friendly fibre-reinforced composites.

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