A Facile Synthesis of ZnCo(2)O(4) Nanocluster Particles and the Performance as Anode Materials for Lithium Ion Batteries

一种简便合成ZnCo(2)O(4)纳米团簇颗粒及其作为锂离子电池负极材料的性能

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Abstract

ABSTRACT: ZnCo(2)O(4) nanocluster particles (NCPs) were prepared through a designed hydrothermal method, with the assistance of a surfactant, sodium dodecyl benzene sulfonate. The crystalline structure and surface morphology of ZnCo(2)O(4) were investigated by XRD, XPS, SEM, TEM, and BET analyses. The results of SEM and TEM suggest a clear nanocluster particle structure of cubic ZnCo(2)O(4) (~100 nm in diameter), which consists of aggregated primary nanoparticles (~10 nm in diameter), is achieved. The electrochemical behavior of synthesized ZnCo(2)O(4) NCPs was investigated by galvanostatic discharge/charge measurements and cyclic voltammetry. The ZnCo(2)O(4) NCPs exhibit a high reversible capacity of 700 mAh g(-1) over 100 cycles under a current density of 100 mA g(-1) with an excellent coulombic efficiency of 98.9% and a considerable cycling stability. This work demonstrates a facile technique designed to synthesize ZnCo(2)O(4) NCPs which show great potential as anode materials for lithium ion batteries.

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