From Antiaromatic Norcorrolatonickel(II) to Aromatic and Nonaromatic Zwitterions: Innocent Ligands with Unbalanced Charge of the Core

从反芳香性降钙素(II)到芳香性和非芳香性两性离子:核心电荷不平衡的无辜配体

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Abstract

A three-component reaction of antiaromatic meso-mesityl-3-nitronorcorrolatonickel(II) 1-NO(2) with dialkyl acetylenedicarboxylate and PBu(3) yields aromatic zwitterionic corrole nickel(II) complexes 3-R with one of the meso-substituents comprising a positively charged tributyl phosphonium group and negatively charged coordination core. Reaction of 1-NO(2) with PBu(3) alone resulted in a nonaromatic chiral adduct 5 of a zwitterionic phlorine character with a -PBu(3)(+) group at a pyrrole β-position.

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