Intercepting Wacker intermediates with arenes: C-H functionalization and dearomatization

利用芳烃截获Wacker中间体:CH官能化和去芳构化

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Abstract

An intramolecular cyclization cascade reaction has been developed utilizing a high valent palladium intermediate that generates a carbon-carbon and carbon-oxygen bond in a single transformation. This method provides rapid access to highly functionalized tricyclic scaffolds, including spirocyclic cyclohexadienones. Good yields and mild conditions are reported with high tolerance toward oxygen and water.

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